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Origami Inspired Self-assembly of Patterned and Reconfigurable Particles
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Self-assembly of 10-microm-sized objects into ordered three-dimensional arrays.

T D Clark1, J Tien, D C Duffy

  • 1Department of Chemistry and Chemical Biology, Harvard University, 12 Oxford Street, Cambridge, Massachusetts 02138, USA.

Journal of the American Chemical Society
|August 2, 2001
PubMed
Summary

Researchers demonstrate self-assembly of microscale metal plates into ordered 3D arrays using capillary forces. This method enables fabrication of complex microstructures by controlling plate properties and assembly conditions.

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Area of Science:

  • Materials Science
  • Nanotechnology
  • Surface Chemistry

Background:

  • Fabricating ordered three-dimensional microstructures is challenging.
  • Controlling self-assembly at the microscale is crucial for advanced materials and devices.

Purpose of the Study:

  • To describe the self-assembly of polyhedral metal plates into ordered 3D arrays.
  • To investigate the role of capillary interactions in driving microscale self-assembly.
  • To explore methods for creating complex, open 3D microstructures.

Main Methods:

  • Fabrication of microscale polyhedral metal plates using photolithography and electrodeposition.
  • Surface functionalization with hydrophobic/hydrophilic self-assembled monolayers (SAMs).
  • Inducing self-assembly in water via capillary interactions with a liquid prepolymer adhesive.

Main Results:

  • Achieved highly ordered, three-dimensional arrays of metal plates (10-30 microm).
  • Demonstrated control over aggregate morphology by varying plate size and surface patterning.
  • Created mechanically stable aggregates and fully open 3D microstructures via sacrificial etching.

Conclusions:

  • Capillary interactions effectively drive mesoscale self-assembly in the 10-microm regime.
  • This approach offers new possibilities for fabricating complex 3D microstructures.
  • Validated a novel method for creating ordered microscale assemblies.