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Dynamic scaling and freezing criteria in quasi-two-dimensional dispersions
R Pesché1, M Kollmann, G Nägele
1Department of Chemical Engineering, University of Delaware, Newark, Delaware 19716, USA.
Physical Review. E, Statistical, Nonlinear, and Soft Matter Physics
|December 12, 2001
Abstract:
We report on a Brownian dynamics simulation study of quasi-two-dimensional dispersions of colloidal spheres interacting by long-range electrostatic and dipolar magnetic forces. The calculated dynamic correlation functions are shown to obey dynamic scaling in terms of a characteristic relaxation time related to the mean particle distance and, due to hydrodynamic interactions, to the particle size. The dynamical freezing criterion of Löwen [Phys. Rev. E 53, R29 (1996)] is shown to be equivalent to a two-dimensional static freezing criterion.