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Designed layer assembly: a three-dimensional framework with 74% extra-framework volume by connection of infinite

T J Prior1, D Bradshaw, S J Teat

  • 1Department of Chemistry, University of Liverpool, Liverpool, UK L69 7ZD.

Chemical Communications (Cambridge, England)
|March 18, 2003
PubMed
Summary

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Researchers created a novel framework-structured solid using a honeycomb network and two distinct ligands. This coordination polymer exhibits a high 74% extra-framework volume, indicating significant potential for applications.

Area of Science:

  • Materials Science
  • Chemistry

Background:

  • Coordination polymers are versatile materials with tunable properties.
  • Designing frameworks with high porosity is crucial for various applications.

Purpose of the Study:

  • To synthesize a novel coordination polymer with a high extra-framework volume.
  • To explore the predictable assembly of honeycomb networks using distinct ligands.

Main Methods:

  • Utilized predictable linking of a honeycomb network.
  • Employed two distinct connecting ligands for framework construction.

Main Results:

  • Successfully prepared a framework-structured solid.
  • Achieved a significant 74% extra-framework volume within the coordination polymer.

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Conclusions:

  • The study demonstrates a viable strategy for creating highly porous coordination polymers.
  • The designed material holds promise for applications requiring large accessible volumes.