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Updated: Jun 29, 2026

Direct Imaging of Laser-driven Ultrafast Molecular Rotation
Published on: February 4, 2017
Rescattering double ionization of D2 and H2 by intense laser pulses
A S Alnaser1, T Osipov, E P Benis
1J. R. Macdonald Laboratory, Physics Department, Kansas State University, Manhattan, Kansas 66506, USA.
Abstract:
We have measured momentum spectra and branching ratios of charged ionic fragments emitted in the double ionization of D2 (and H2) molecules by short intense laser pulses. We find high-energy coincident D+ (and H+) ion pairs with kinetic energy releases between 8 and 19 eV which appear for linearly polarized light but are absent for circularly polarized light. The dependence on the polarization, the energy distributions of the ions, and the dependence on laser intensity of yield ratios lead us to interpret these ion pairs as due to a rescattering mechanism for the double ionization. A quantitative model is presented which accounts for the major features of the data.
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