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Direct Imaging of Laser-driven Ultrafast Molecular Rotation
Published on: February 4, 2017
Observation of enhanced field-free molecular alignment by two laser pulses
Christer Z Bisgaard1, Mikael D Poulsen, Emmanuel Péronne
1Department of Physics and Astronomy, University of Aarhus, 8000 Arhus C, Denmark.
Physical Review Letters
|June 1, 2004
Abstract:
We show experimentally that field-free alignment of iodobenzene molecules, induced by a single, intense, linearly polarized 1.4-ps-long laser pulse, can be strongly enhanced by dividing the pulse into two optimally synchronized pulses of the same duration. For a given total energy of the two-pulse sequence the degree of alignment is maximized with an intensity ratio of 1:3 and by sending the second pulse near the time where the alignment created by the first pulse peaks.
