Wide spectral range third-order autocorrelator based on ultrafast nonresonant nonlinear refraction

We demonstrate a simple scheme for a wide spectral range, third-order autocorrelator based on ultrafast nonlinear Kerr-type refraction. The technique was successfully used to characterize high-energy ultrashort pulses at 1550 and 1300 nm, where the pulse's shape and width are two of the most critical parameters. Because of its simplicity, this technique is also a powerful tool for the optimization of high-power chirped-pulse amplified laser systems, in which slight misalignment of the stretcher-compressor gratings can lead to spatiotemporal pulse distortions. In addition, it can be extended to low-power mode-locked oscillators.