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Updated: Aug 17, 2026

Direct Imaging of Laser-driven Ultrafast Molecular Rotation
Published on: February 4, 2017
Compression of attosecond harmonic pulses by extreme-ultraviolet chirped mirrors
Anne-Sophie Morlens1, Philippe Balcou, Philippe Zeitoun
1Laboratoire Optique Appliquée, Ecole Nationale Supérieure de Techniques Avancées, Centre National de la Recherche Scientifique, Unité Mixte de Recherche 7639, Chemin de la Hunière, F-91761 Palaiseau, France. Anne-Sophie.Morlens@ensta.fr
Abstract:
In the race toward attosecond pulses, for which high-order harmonics generated in rare gases are the best candidates, both the harmonic spectral range and the spectral phase have to be controlled. We demonstrate that multilayer extreme-ultraviolet chirped mirrors can be numerically optimized and designed to compensate for the intrinsic harmonic chirp that was recently discovered and that is responsible for temporal broadening of pulses. A simulation shows that an optimized mirror is capable of compressing the duration from approximately 260 to 90 as. This new technique is an interesting solution because of its ability to cover a wider spectral range than other technical devices that have already been proposed to overcome the chirp of high harmonics.
