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Updated: Aug 11, 2026

Novel Techniques for Observing Structural Dynamics of Photoresponsive Liquid Crystals
Published on: May 29, 2018
Ring-resonator-based frequency-domain optical activity measurements of a chiral liquid
1The Rowland Institute at Harvard, Harvard University, Cambridge, Massachusetts 02142, USA. vollmer@rowland.harvard.edu
Abstract:
Chiral liquids rotate the plane of polarization of linearly polarized light and are therefore optically active. Here we show that optical rotation can be observed in the frequency domain. A chiral liquid introduced in a fiber-loop ring resonator that supports left and right circularly polarized modes gives rise to relative frequency shifts that are a direct measure of the liquid's circular birefringence and hence of its optical activity. The effect is in principle not diminished if the circumference of the ring is reduced. The technique is similarly applicable to refractive index and linear birefringence measurements.
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