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Updated: Aug 9, 2026

09:53
Predicting Catalyst Extrudate Breakage Based on the Modulus of Rupture
Published on: May 13, 2018
Geometry-induced pulse instability in microdesigned catalysts: the effect of boundary curvature
L Qiao1, I G Kevrekidis, C Punckt
1Department of Chemical Engineering, Princeton University, Princeton, NJ 08544, USA.
Abstract:
We explore the effect of boundary curvature on the instability of reactive pulses in the catalytic oxidation of on microdesigned Pt catalysts. Using ring-shaped domains of various radii, we find that the pulses disappear (decollate from the inert boundary) at a turning point bifurcation, and we trace this boundary in both physical and geometrical parameter space. These computations corroborate experimental observations of pulse decollation.
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