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Updated: Jul 16, 2026

Experimental Methods for Spin- and Angle-Resolved Photoemission Spectroscopy Combined with Polarization-Variable Laser
Published on: June 28, 2018
Photoinduced metallic state mediated by spin-charge separation in a one-dimensional organic Mott insulator
H Okamoto1, H Matsuzaki, T Wakabayashi
1Department of Advanced Materials Science, University of Tokyo, Kashiwa, 277-8561, Japan.
Abstract:
Charge dynamics in a one-dimensional (1D) Mott insulator was investigated by fs pump-probe reflection spectroscopy on an organic charge-transfer compound, bis(ethylenedithio)tetrathiafulvalene-difluorotetracyanoquinodimethane (ET-F2TCNQ). The analyses of the transient reflectivity changes demonstrate that low-energy spectral weight induced by photocarrier doping is concentrated on a Drude component being independent of the doping density, and midgap state is never formed. Such phenomena can be explained by the concept of spin-charge separation characteristic of 1D correlated electron systems.
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