Related Experiment Video
Updated: Jul 10, 2026

High Resolution Phonon-assisted Quasi-resonance Fluorescence Spectroscopy
Published on: June 28, 2016
Laser-induced nonlinear response in photoassisted resonant electronic transport
Inés Urdaneta1, Arne Keller, Osman Atabek
1Laboratoire de Photophysique Moléculaire du CNRS, Université Paris-Sud, 91405 Orsay Cedex, France.
Abstract:
We consider an extension of our previous model for photoassisted electron transport in molecular and atomic junctions to the study of nonlinear processes, induced by a laser field, that are strongly influenced by a resonant level structure associated with the material structure between the two metal electrodes. Using a Floquet transformation to include the radiation field, we calculate the stationary Landauer current as a function of the intensity and frequency of the laser. The emphasis in this work is in the description of the interplay between the optical response of the junction and its transport properties. Our results may be then of importance in understanding the response of molecular junctions to multiphoton excitations, a regime where nonlinearities are dominant.

