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Attosecond electron dynamics.

Matthias F Kling¹, Marc J J Vrakking

¹FOM Institute for Atomic and Molecular Physics, 1098 SJ Amsterdam, The Netherlands. m.vrakking@amolf.nl

Annual Review of Physical Chemistry

|November 23, 2007

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Attosecond science, using ultrashort laser pulses, now allows detailed studies of electron dynamics in atoms and molecules. This emerging field reveals fundamental insights into multielectron interactions in physics and chemistry.

Area of Science:

Physics
Chemistry
Quantum mechanics

Background:

Attosecond science is an emerging field utilizing ultrashort laser pulses.
Understanding electron dynamics is crucial in atomic and molecular systems.

Purpose of the Study:

To review the state of the art in attosecond science.
To highlight recent advancements and applications in studying electron dynamics.

Main Methods:

Generation and characterization of attosecond laser pulses.
Pump-probe experiments with isolated attosecond pulses.
Interference experiments with attosecond pulse trains.
Waveform-controlled electron dynamics using ultrashort laser pulses.

Main Results:

Related Experiment Videos

Demonstrated subcycle time dependence of multiphoton ionization.
Extracted amplitude and phase information for electronic wave functions.
Controlled electron dynamics in D(2)(+) molecular ions on attosecond timescales.

Conclusions:

Attosecond science has reached a level of sophistication for detailed investigations.
The field enables deeper understanding of multielectron dynamics in physics and chemistry.