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Periodically poled BaMgF(4) for ultraviolet frequency generation.

S C Buchter, T Y Fan, V Liberman

    Optics Letters
    |December 1, 2007
    PubMed
    Summary

    Ferroelectric domain inversion is now possible in Barium Magnesium Fluoride (BaMgF4). This material shows exceptional transparency and stability, enabling advanced nonlinear optical applications at shorter wavelengths.

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    Area of Science:

    • Materials Science
    • Nonlinear Optics
    • Solid-State Physics

    Background:

    • Barium Magnesium Fluoride (BaMgF4) is a crystalline material with potential nonlinear optical properties.
    • Achieving ferroelectric domain inversion is crucial for applications like quasi-phase-matching in nonlinear optics.
    • Previous research has not demonstrated domain inversion in BaMgF4.

    Purpose of the Study:

    • To demonstrate ferroelectric domain inversion in BaMgF4.
    • To evaluate the optical transparency and laser-induced damage threshold of BaMgF4 at deep ultraviolet (DUV) wavelengths.
    • To explore the potential of BaMgF4 for nonlinear optical frequency conversion.

    Main Methods:

    • Ferroelectric domain inversion was induced in BaMgF4 crystals.
    • Optical transmission measurements were performed down to <140 nm.

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  • BaMgF4 samples were irradiated with 157-nm laser pulses to assess laser-induced damage threshold.
  • Main Results:

    • Ferroelectric domain inversion was successfully demonstrated in BaMgF4.
    • The material exhibits transparency below 140 nm.
    • BaMgF4 showed no change in transmission after >1.1x10^9 shots at 2 mJ/cm^2 per pulse at 157 nm.
    • First-order quasi-phase-matched generation of 157 nm is predicted using grating periods as long as 1.5 μm.

    Conclusions:

    • BaMgF4 is a promising material for nonlinear optical applications.
    • Its demonstrated domain invertibility and DUV transparency/stability surpass existing crystalline materials.
    • BaMgF4 could enable shorter-wavelength chi((2)) frequency-mixing processes.