Related Experiment Video
Updated: Jul 9, 2026

Direct Imaging of Laser-driven Ultrafast Molecular Rotation
Published on: February 4, 2017
Intracavity second-harmonic and sum-frequency generation with a laser-diode-pumped multitransition-oscillation
1Department of Applied Physics, School of Engineering, Tokai University, 1117 Kitakaname, Hiratsuka, Kanagawa 259-1292 Japan.
Abstract:
Efficient simultaneous intracavity second-harmonic and sum-frequency generation that is free from irregular large amplitude fluctuations (the so-called green problem) is achieved with a laser-diode-pumped LiNdP(4)O(12) (LNP) laser with a type II phase-matching KTiOPO(4) crystal. Observed frequency-mixing operations result from the simultaneous single-frequency oscillations on different transitions that arise from the wide fluorescence linewidth in a stoichiometric LNP laser that possesses inherently high Nd concentrations. Sum-frequency generation has been shown to arise from the interaction of oscillating longitudinal modes that belong to different transitions. A promising application to coherent terahertz-wave radiation by use of photomixers is proposed.

