High-efficiency blue generation by frequency doubling of femtosecond pulses in a thick nonlinear crystal

We have demonstrated highly efficient frequency doubling of femtosecond pulses in a thick, noncritically phase-matched KNbO(3) crystal under conditions of large group-velocity mismatch. At low power we observed a slope efficiency of ~300% nJ (-1) for harmonic conversion, and at higher powers we generated 170 mW of second-harmonic blue output for 300 mW of input light. Furthermore, we have shown that the focusing dependence for our conditions of large group-velocity mismatch is considerably different from that obtained for frequency doubling of continuous-wave light. We have also demonstrated that one can tune the spectral width of the generated blue light by varying the focusing conditions.