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Determination of the Excitation and Coupling Rates Between Light Emitters and Surface Plasmon Polaritons
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Photonic-plasmonic scattering resonances in deterministic aperiodic structures.

Ashwin Gopinath1, Svetlana V Boriskina, Ning-Ning Feng

  • 1Department of Electrical and Computer Engineering, Boston University, Boston, Massachusetts 02215-2421, USA.

Nano Letters
|July 24, 2008
PubMed
Summary

Deterministic aperiodic gold nanoparticle arrays exhibit broad plasmonic resonances across the visible spectrum. This broadband plasmonic enhancement from engineered nanoparticle lattices impacts nanodevice design.

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Area of Science:

  • Plasmonics and Nanophotonics
  • Materials Science

Background:

  • Plasmonic lattices offer tunable optical properties.
  • Aperiodic order presents unique scattering phenomena.

Purpose of the Study:

  • Investigate scattering properties of aperiodic plasmonic lattices.
  • Explore broadband plasmonic resonances in deterministic nanoparticle arrays.

Main Methods:

  • Experimental dark-field scattering spectroscopy.
  • Electrodynamics calculations and generalized Mie theory.
  • Electron-beam lithography for fabricating gold nanoparticle lattices.

Main Results:

  • Aperiodic gold nanoparticle arrays show broad plasmonic resonances across the visible spectrum.
  • Far-field diffractive coupling creates photonic-plasmonic scattering modes.
  • Experimental results are supported by accurate scattering simulations.

Conclusions:

  • Deterministic aperiodic lattices enable broadband plasmonic enhancement.
  • Engineered nanoparticle arrays have significant potential for novel nanodevices.