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Related Concept Videos

X-ray Imaging01:24

X-ray Imaging

German physicist Wilhelm Röntgen (1845–1923) was experimenting with electrical current when he discovered that a mysterious and invisible "ray" would pass through his flesh but leave an outline of his bones on a screen coated with a metal compound. In 1895, Röntgen made the first durable record of the internal parts of a living human: an "X-ray" image (as it came to be called) of his wife’s hand. Scientists worldwide quickly began their own experiments with X-rays, and by 1900, X-ray was widely...
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X-ray Crystallography

The size of the unit cell and the arrangement of atoms in a crystal may be determined from measurements of the diffraction of X-rays by the crystal, termed X-ray crystallography.
Diffraction
Diffraction is the change in the direction of travel experienced by an electromagnetic wave when it encounters a physical barrier whose dimensions are comparable to those of the wavelength of the light. X-rays are electromagnetic radiation with wavelengths about as long as the distance between neighboring...

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Measurements of Long-range Electronic Correlations During Femtosecond Diffraction Experiments Performed on Nanocrystals of Buckminsterfullerene
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Measuring temporal speckle correlations at ultrafast x-ray sources.

C Gutt1, L-M Stadler, A Duri

  • 1Hasylab at DESY, Hamburg, Germany. christian.gutt@desy.de

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|January 9, 2009
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Summary

Researchers developed a novel method using photon statistics to analyze speckle patterns from coherent diffraction data. This technique extracts the intermediate scattering function for ultrafast correlation spectroscopy at X-ray free-electron laser sources.

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Area of Science:

  • X-ray science
  • Photonics
  • Materials science

Background:

  • Coherent diffraction imaging (CDI) provides structural information.
  • Extracting dynamic information from CDI is challenging.
  • Ultrafast processes require advanced spectroscopic techniques.

Purpose of the Study:

  • To present a new method for extracting the intermediate scattering function (ISF) from coherent diffraction patterns.
  • To demonstrate the equivalence of this new method to conventional techniques.
  • To enable correlation spectroscopy on ultrafast timescales.

Main Methods:

  • Analysis of speckle patterns in coherent diffraction data using photon statistics.
  • Utilizing 2D detectors for data acquisition.
  • Comparison with the intensity autocorrelation function method.

Main Results:

  • Successfully extracted the intermediate scattering function.
  • Demonstrated that the photon statistics approach yields equivalent information to the intensity autocorrelation function.
  • Established a viable method for ultrafast dynamics studies.

Conclusions:

  • The novel photon statistics method offers a powerful tool for analyzing ultrafast dynamics.
  • This approach is suitable for X-ray free-electron laser (XFEL) sources.
  • Opens new avenues for correlation spectroscopy at unprecedented timescales.