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Related Experiment Video

Updated: Jun 23, 2026

An Experimental Protocol for Femtosecond NIR/UV - XUV Pump-Probe Experiments with Free-Electron Lasers
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An Experimental Protocol for Femtosecond NIR/UV - XUV Pump-Probe Experiments with Free-Electron Lasers

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Picosecond time-resolved laser pump/X-ray probe experiments using a gated single-photon-counting area detector.

T Ejdrup1, H T Lemke, K Haldrup

  • 1Danish National Research Foundation Centre for Molecular Movies, Niels Bohr Institute, University of Copenhagen, Universitetsparken 5, 2100 Copenhagen Ø, Denmark. ejdrup@fys.ku.dk

Journal of Synchrotron Radiation
|April 28, 2009
PubMed
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This study demonstrates a novel method for achieving 60 picosecond time-resolution in X-ray experiments using a gated PILATUS detector. This advancement enables pulse duration-limited data collection without mechanical choppers.

Area of Science:

  • Materials Science
  • Physics
  • X-ray Science

Background:

  • Time-resolved X-ray experiments are crucial for studying dynamic processes.
  • Conventional methods often rely on mechanical choppers, limiting time resolution.
  • Recent advancements in X-ray detectors offer new possibilities for high-resolution studies.

Purpose of the Study:

  • To demonstrate the novel use of a PILATUS detector for time-resolved pump/probe X-ray experiments.
  • To achieve X-ray pulse duration limited time-resolution at the Advanced Photon Source (APS).
  • To showcase the capability of a gated PILATUS detector in selective X-ray pulse detection.

Main Methods:

  • Utilized a gated PILATUS detector at the Advanced Photon Source (APS).
  • Operated the detector in a 24 bunch mode for selective X-ray pulse detection.

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  • Conducted experiments on polycrystalline organic thin films of alpha-perylene.

    • Main Results:

    • Demonstrated the capability of the gated PILATUS detector to achieve X-ray pulse duration limited time-resolution.
    • Achieved a time-resolution of 60 picoseconds (ps).
    • Successfully recorded time-resolved data without employing a mechanical chopper array.

    Conclusions:

    • The gated PILATUS detector enables X-ray pulse duration limited time-resolution in pump/probe experiments.
    • This method offers a significant advancement for high-resolution X-ray studies.
    • It is the first demonstration of such data acquisition using an area detector without mechanical choppers.