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Direct Imaging of Laser-driven Ultrafast Molecular Rotation
Published on: February 4, 2017
Ultrabroadband 50-130 THz pulses generated via phase-matched difference frequency mixing in LiIO(3)
Optics Express
|June 18, 2009
Abstract:
We report the generation of ultrabroadband pulses spanning the 50-130 THz frequency range via phase-matched difference frequency mixing within the broad spectrum of sub-10 fs pulses in LiIO(3). Model calculations reproduce the octave-spanning spectra and predict few-cycle THz pulse durations less than 20 fs. The broad applicability of this scheme is demonstrated with 9-fs pulses from a Ti:sapphire oscillator and with 7-fs amplified pulses from a hollow fiber compressor as pump sources.
