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Direct Imaging of Laser-driven Ultrafast Molecular Rotation
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Generation of 8.5-fs pulses at 1.3 microm for ultrabroadband pump-probe spectroscopy

Daniele Brida1, Stefano Bonora, Cristian Manzoni

  • 1Dipartimento di Fisica, Politecnico di Milano, Piazza Leonardo da Vinci 32, 20133 Milano, Italy.

Optics Express
|August 6, 2009
PubMed

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A pulse is a short burst of radio waves distributed over a range of frequencies that simultaneously excites all the nuclei in the sample. Upon passing a radio frequency pulse along the x-axis, the nuclei absorb energy corresponding to their Larmor frequencies and achieve resonance. This shifts the net magnetization vector from the z-axis toward the transverse plane. This angle of rotation of the magnetization vector, or the flip angle, is proportional to the duration and intensity of the pulse.