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Materials like iron, nickel, and cobalt consist of magnetic domains, within which the magnetic dipoles are arranged parallel to each other. The magnetic dipoles are rigidly aligned in the same direction within a domain by quantum mechanical coupling among the atoms. This coupling is so strong that even thermal agitation at room temperature cannot break it. The result is that each domain has a net dipole moment. However, some materials have weaker coupling, and are ferromagnetic at lower...
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Fermi-surface shrinking and interband coupling in iron-based pnictides.

L Ortenzi1, E Cappelluti, L Benfatto

  • 1Dipartimento di Fisica, Università La Sapienza, 00185 Rome, Italy.

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|August 8, 2009
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Summary

Measurements of LaFePO revealed shrinking Fermi pockets, indicating an energy shift in electronic bands. This suggests strong particle-hole asymmetry and dominant interband scattering in pnictides.

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Area of Science:

  • Condensed Matter Physics
  • Materials Science
  • Solid-State Physics

Background:

  • Recent de Haas-van Alphen oscillation measurements in LaFePO indicate discrepancies between experimental Fermi surfaces and first-principle calculations.
  • These discrepancies suggest a potential energy shift in the hole and electron bands relative to local-density approximations.

Purpose of the Study:

  • To investigate the cause of the observed shrinking of Fermi pockets in LaFePO.
  • To explore the role of particle-hole asymmetry in the electronic band structure of pnictides.
  • To provide experimental evidence for interband scattering mechanisms.

Main Methods:

  • Analysis of de Haas-van Alphen oscillation data for LaFePO.
  • Comparison of experimental Fermi surface measurements with theoretical calculations.
  • Theoretical modeling to account for band shifts and particle-hole asymmetry.

Main Results:

  • The study demonstrates that the observed shrinking of Fermi pockets is a natural consequence of strong particle-hole asymmetry in the electronic bands of LaFePO.
  • Calculations incorporating this asymmetry successfully explain the experimental observations.
  • The findings provide indirect experimental evidence for significant interband scattering.

Conclusions:

  • The strong particle-hole asymmetry of electronic bands in pnictides is a key factor influencing Fermi surface properties.
  • Interband scattering plays a dominant role in the electronic transport of these materials.
  • Discrepancies between theory and experiment in LaFePO can be reconciled by considering band asymmetry and scattering effects.