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Updated: Jun 20, 2026

Direct Imaging of Laser-driven Ultrafast Molecular Rotation
Published on: February 4, 2017
Direct spatiotemporal measurements of accelerating ultrashort Bessel-type light bullets
Heli Valtna-Lukner1, Pamela Bowlan, Madis Lõhmus
1Institute of Physics, University of Tartu, Riia 142, Tartu, 51014 Estonia. heli.lukner@ut.ee
Abstract:
We measure the spatiotemporal field of ultrashort pulses with complex spatiotemporal profiles using the linear-optical, interferometric pulse-measurement technique SEA TADPOLE. Accelerating and decelerating ultrashort, localized, nonspreading Bessel-X wavepackets were generated from a approximately 27 fs duration Ti:Sapphire oscillator pulse using a combination of an axicon and a convex or concave lens. The wavefields are measured with approximately 5 microm spatial and approximately 15 fs temporal resolutions. Our experimental results are in good agreement with theoretical calculations and numerical simulations.

