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Updated: Jun 20, 2026

Flame Experiments at the Advanced Light Source: New Insights into Soot Formation Processes
Published on: May 26, 2014
Asynchronous optical sampling: a new combustion diagnostic for potential use in turbulent, high-pressure flames
Abstract:
Asynchronous optical sampling (ASOPS) is a pump-probe method that has strong potential for use in turbulent, high-pressure flames. We show that rapid measurement of species number density can be achieved by maintaining a constant beat frequency between the mode-locking frequencies of the pump and probe lasers. We also describe the instrumental timing parameters for ASOPS and consider the optimization of these parameters. Measurement of the nanosecond decay for electronically excited sodium in an atmospheric flame demonstrates the viability of the ASOPS technique in highly quenched flame environments.
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