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Published on: March 24, 2019
Spin-lattice coupling, frustration, and magnetic order in multiferroic RMnO3
X Fabrèges1, S Petit, I Mirebeau
1Laboratoire Léon Brillouin, CEA-CNRS, CE-Saclay, 91191 Gif-sur-Yvette, France.
Strong magnetoelastic coupling in frustrated multiferroic hexagonal RMnO3 compounds is linked to Mn ion position. This critical atomic arrangement dictates magnetic structure and spin wave behavior across various R ions and temperatures.
Area of Science:
- Condensed matter physics
- Materials science
- Magnetism
Background:
- Frustrated multiferroic hexagonal compounds (RMnO3) exhibit complex magnetic and structural properties.
- Understanding the interplay between magnetism and lattice structure is crucial for these materials.
Purpose of the Study:
- To investigate the relationship between atomic positions, magnetic structure, and spin wave dynamics in RMnO3 compounds.
- To identify the key structural parameter governing magnetoelastic coupling in this material family.
Main Methods:
- High-resolution neutron diffraction experiments.
- Inelastic neutron scattering experiments.
Main Results:
- Evidence of strong magnetoelastic coupling across the RMnO3 family.
- Correlation established between atomic positions, magnetic structure, and spin wave nature.
- Mn ion position relative to 1/3 in the unit cell identified as a critical parameter.
Conclusions:
- The position of Mn ions is a key determinant of the coupling between Mn triangular planes in RMnO3.
- This finding provides a unified understanding of magnetic and structural properties in these frustrated multiferroics.
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