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Measurement of Ultrafast Vibrational Coherences in Polyatomic Radical Cations with Strong-Field Adiabatic Ionization
Published on: August 6, 2018
Classical aspects in above-threshold ionization with a midinfrared strong laser field
1State Key Laboratory of Magnetic Resonance and Atomic and Molecular Physics, Wuhan Institute of Physics and Mathematics, Chinese Academy of Sciences, Wuhan 430071, China.
We observed a new low-energy structure in photoelectron spectra from above-threshold ionization (ATI) of noble gases using mid-infrared lasers. This finding challenges simple theories and highlights the role of electron-ion interactions in long-wavelength ATI.
Area of Science:
- Atomic Physics
- Quantum Mechanics
- Laser Physics
Background:
- Above-threshold ionization (ATI) is a fundamental process in strong-field physics.
- Existing theoretical models, like the simple-man theory, do not fully explain experimental observations in all regimes.
- Mid-infrared lasers offer unique parameters for exploring ATI phenomena.
Purpose of the Study:
- To investigate high-resolution photoelectron energy spectra of noble gas atoms under high-intensity ATI.
- To explore the influence of mid-infrared wavelengths on ATI spectra.
- To understand unexpected structures observed in the low-energy portion of the spectra.
Main Methods:
- High-resolution photoelectron spectroscopy.
- High-intensity above-threshold ionization (ATI) experiments.
- Semiclassical model calculations.
Main Results:
- High-resolution photoelectron energy spectra of noble gas atoms were obtained using mid-infrared laser wavelengths.
- An unexpected low-energy structure was observed in the spectra, contradicting predictions from the simple-man theory.
- Semiclassical model calculations successfully reproduced the experimental feature.
Conclusions:
- The observed low-energy structure in ATI spectra is attributed to the Coulomb interaction between the outgoing electron and the parent ion.
- This Coulomb interaction plays a significant role in shaping photoelectron spectra at long laser wavelengths.
- The findings necessitate refinements to theoretical models for describing ATI processes, particularly in the long-wavelength regime.
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