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Three-dimensional jamming and flows of soft glassy materials
G Ovarlez1, Q Barral, P Coussot
1Université Paris Est, Laboratoire Navier, LMSGC (CNRS-ENPC-LCPC), 77420 Champs sur Marne, France. guillaume.ovarlez@lcpc.fr
Nature Materials
|January 12, 2010
Summary
Soft glassy materials jam from liquid to solid states. Experiments reveal they unjam in all directions simultaneously, behaving like simple liquids under secondary flow, crucial for geophysical and industrial applications.
Area of Science:
- Physics
- Materials Science
- Rheology
Background:
- Disordered dense systems like foams, gels, and suspensions exhibit a jamming transition.
- These soft glassy materials share structural similarities with conventional glasses.
- Their nonlinear rheological behavior and microscopic origins remain poorly understood despite significant applications.
Purpose of the Study:
- To develop a simple three-dimensional continuum description for soft glassy materials.
- To investigate the jamming transition and rheological properties of these systems.
- To elucidate the microscopic origins of their complex flow behavior.
Main Methods:
- Conducted two original experiments to probe the mechanical response of soft glassy materials.
- Applied controlled shear flow in specific directions.
- Observed system behavior under secondary flow conditions and across different directions.
Main Results:
- Demonstrated that soft glassy materials unjam simultaneously in all spatial directions, lacking directional yield resistance.
- Identified the jamming criterion as analogous to the plasticity criterion in solids.
- Observed liquid-like behavior in directions orthogonal to the main flow, with shear rate-dependent viscosity.
Conclusions:
- A simple 3D continuum model can describe the behavior of soft glassy materials.
- The jamming transition is isotropic, and the plasticity criterion governs it.
- Shear-induced structural relaxation influences viscosity, mirroring temperature and density effects in other glasses.
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