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V G Kravets1, G Zoriniants, C P Burrows

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We developed composite plasmonic nanostructures that significantly boost light-matter interactions. These structures show a 43-fold increase in fluorescence, enabling advanced applications in sensing and optical manipulation.

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Area of Science:

  • Plasmonics
  • Nanophotonics
  • Optical Engineering

Background:

  • Plasmonic nanostructures are crucial for manipulating light at the nanoscale.
  • Cascaded enhancement of electromagnetic fields is key for improving optical phenomena.
  • Controlling field localization in composite nanostructures remains a challenge.

Purpose of the Study:

  • To design and investigate composite plasmonic nanostructures for cascaded electromagnetic field enhancement.
  • To quantify the fluorescence enhancement achieved by these novel nanostructures.
  • To explore potential applications in sensing and optical manipulation.

Main Methods:

  • Fabrication of two-tier composite nanostructures (small nanodisc over larger disk).
  • Coating nanostructures with visible-light fluorophores.
  • Probing optical properties using scanning confocal microscopy and fluorescence measurements.

Main Results:

  • Observed a significant 43 ± 5-fold increase in far-field fluorescence signal for composite nanostructures compared to individual nanodiscs.
  • Demonstrated cascaded enhancement of electromagnetic fields at optical frequencies.
  • Validated the effectiveness of the designed nanostructures for signal amplification.

Conclusions:

  • Composite plasmonic nanostructures effectively achieve cascaded electromagnetic field enhancement.
  • The observed fluorescence enhancement opens possibilities for advanced optical applications.
  • These nanostructures show promise for applications in field concentration, optical manipulation, and chemical/biological sensing.