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Dynamical coupling and separation of multiple degrees of freedom in a photoexcited double-exchange system
Y Kanamori1, H Matsueda, S Ishihara
1Department of Physics, Tohoku University, Sendai 980-8578, Japan.
Abstract:
We present a theory of ultrafast photoinduced dynamics in a spin-charge coupled system, motivated by pump-probe experiments in perovskite manganites. A microscopic picture for multiple dynamics in spin and charge degrees is examined. Real-time simulations are carried out by two complimentary methods. Our calculation demonstrates that electron motion governs a short-time scale where charge and spin dynamics are combined strongly, while, in a long-time scale controlled by spin relaxation, the charge sector does not follow the remarkable change in the spin sector. The present results are in contrast to a conventional double-exchange picture in equilibrium states.
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