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Updated: Aug 12, 2026

Direct Imaging of Laser-driven Ultrafast Molecular Rotation
Published on: February 4, 2017
Generation of sub-50-fs vacuum ultraviolet pulses by four-wave mixing in argon
Marcus Beutler1, Masood Ghotbi, Frank Noack
1Max-Born-Institute for Nonlinear Optics and Ultrafast Spectroscopy, Max-Born-Strasse 2a, 12489 Berlin, Germany. beutler@mbi-berlin.de
Abstract:
We report on the generation of femtosecond pulses at 160 nm with energies up to 240 nJ at 1 kHz repetition rate and sub-50-fs pulse duration. This pulse energy is a 1-order-of-magnitude improvement compared with previous sub-100-fs sources in this wavelength range. The pulses are generated by four-wave difference-frequency mixing process between the fundamental of a Ti:sapphire laser and its third harmonic in argon. Pulse duration measurements are achieved by pump-probe ionization of Xe gas providing the cross correlation between the fifth harmonic and the fundamental.

