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Updated: Jun 12, 2026

Generation and Coherent Control of Pulsed Quantum Frequency Combs
Published on: June 8, 2018
Coherent control of angular momentum transfer in resonant two-photon light-matter interaction
D A Malik1, A V Kimel, A Kirilyuk
1Radboud University Nijmegen, Institute for Molecules and Materials, P.O. Box 9010, NL-6500 GL Nijmegen, The Netherlands.
Abstract:
We show experimentally and theoretically that a polarization-shaped femtosecond laser pulse with a zero net angular momentum creates a net angular momentum in atomic rubidium during resonant two-photon excitation. The necessary conditions for the creation of a nonzero angular momentum as well as the excitation efficiencies are analyzed in the framework of second-order time-dependent perturbation theory.
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