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Updated: Jun 12, 2026

Characterizing Far-infrared Laser Emissions and the Measurement of Their Frequencies
Published on: December 18, 2015
Source for ultrafast continuum infrared and terahertz radiation
Poul B Petersen1, Andrei Tokmakoff
1Department of Chemistry and Chemical Biology, Cornell University, 122 Baker Laboratory, Ithaca, New York 14853-1301, USA. pbp33@cornell.edu
A new method generates high-intensity, polarized mid-infrared and terahertz light using ultrafast laser pulses. This compact source is practical for transient infrared spectroscopy applications.
Area of Science:
- Optics and Photonics
- Laser Physics
- Nonlinear Optics
Background:
- Generating broadband mid-infrared (mid-IR) and terahertz (THz) light is crucial for various spectroscopic applications.
- Existing methods often lack compactness, stability, or sufficient intensity for certain applications.
Purpose of the Study:
- To demonstrate a compact and stable method for generating high-intensity, linearly polarized continuum mid-IR and THz light.
- To utilize nonlinear mixing of ultrafast laser harmonics in air for broadband light generation.
Main Methods:
- Ultrafast femtosecond (fs) laser pulses were used as the primary source.
- Nonlinear mixing of the fundamental, second, and third harmonics of the laser in air via filamentation.
- A compact collinear optical configuration with a delay plate was employed for simplified alignment and enhanced stability.
Main Results:
- Continuous light generation was achieved from <400 cm⁻¹ (12 THz) to >3300 cm⁻¹ (100 THz).
- The generated light is linearly polarized and has high intensity.
- Including the third harmonic in the mixing scheme resulted in a tenfold increase in the generated infrared power.
Conclusions:
- A practical and stable source for generating broadband, high-intensity mid-IR and THz light has been demonstrated.
- The compact design and simplified alignment make this method suitable for widespread adoption.
- This technique is particularly promising for applications in transient infrared spectroscopy.
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