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Effect of Bending on the Electrical Characteristics of Flexible Organic Single Crystal-based Field-effect Transistors
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Solution-processed, high-performance nanoribbon transistors based on dithioperylene.

Wei Jiang1, Yan Zhou, Hua Geng

  • 1Beijing National Laboratory for Molecular Sciences, Key Laboratory of Organic Solids, Institute of Chemistry, Chinese Academy of Sciences (CAS), Beijing 100190, China.

Journal of the American Chemical Society
|December 15, 2010
PubMed
Summary
This summary is machine-generated.

High-performance single-crystalline nanoribbon transistors were fabricated using dithioperylene. The sulfur atoms induced ordered packing, achieving high charge carrier mobility for electronic applications.

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Area of Science:

  • Materials Science
  • Organic Electronics
  • Nanotechnology

Background:

  • Organic field-effect transistors (OFETs) are crucial for flexible electronics.
  • Achieving high charge carrier mobility in organic semiconductors remains a challenge.
  • Molecular design is key to controlling solid-state packing and electronic properties.

Purpose of the Study:

  • To develop solution-processed, high-performance transistors using a novel organic semiconductor.
  • To investigate the impact of sulfur incorporation on molecular packing and charge transport.
  • To explore the potential of dithioperylene-based nanoribbons for electronic applications.

Main Methods:

  • Synthesis of dithioperylene molecules.
  • Fabrication of 1D single-crystalline nanoribbon transistors via solution processing.
  • Characterization of molecular packing using X-ray diffraction (if applicable, otherwise omit).
  • Electrical characterization of transistor performance, including charge carrier mobility measurements.

Main Results:

  • Successfully fabricated solution-processed, 1D single-crystalline nanoribbon transistors from dithioperylene.
  • Demonstrated that incorporating two sulfur atoms into the perylene skeleton promotes a compressed, highly ordered packing mode.
  • Observed S···S interactions guiding the molecular assembly.
  • Achieved high charge carrier mobilities up to 2.13 cm(2) V(-1) s(-1) in individual dithioperylene nanoribbons.

Conclusions:

  • Dithioperylene is a promising organic semiconductor for high-performance electronic devices.
  • The molecular design strategy effectively controls solid-state packing for enhanced charge transport.
  • Solution-processed dithioperylene nanoribbon transistors offer potential for advanced electronic applications.