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Updated: Jun 5, 2026

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Fabrication of Three-Dimensional Graphene-Based Polyhedrons via Origami-Like Self-Folding
Published on: September 23, 2018
Production of extended single-layer graphene
Mingsheng Xu1, Daisuke Fujita, Keisuke Sagisaka
1International Center for Young Scientists, National Institute for Materials Science, 1-2-1 Sengen, Tsukuba, Ibaraki 305-0047, Japan. msxu@zju.edu.cn
ACS Nano
|January 14, 2011
Summary
Researchers developed a low-temperature method to produce large-area single-layer graphene sheets. Carbon atoms from a graphite substrate diffuse through a nickel film, enabling controlled graphene synthesis for scalable applications.
Area of Science:
- Materials Science
- Nanotechnology
- Condensed Matter Physics
Background:
- Graphene exhibits exceptional electronic, optical, and mechanical properties, driving significant research interest.
- Scalable synthesis of high-quality single-layer graphene remains a key challenge for practical applications.
Purpose of the Study:
- To develop a low-temperature method for producing large-area, single-layer graphene films.
- To demonstrate control over graphene thickness and crystal structure during synthesis.
Main Methods:
- Synthesis of single-layer graphene on a nickel (Ni) film deposited on highly oriented pyrolytic graphite (HOPG).
- Heating the Ni/HOPG substrate in a vacuum to facilitate carbon diffusion from HOPG through the Ni template.
- Controlling the amount of carbon atoms available for graphene formation.
Main Results:
- Successfully produced single-layer graphene fully covering a 2 cm ×2 cm substrate at low temperatures.
- Demonstrated that carbon atoms originate from the graphite substrate, diffusing through the nickel film.
- Achieved controlled thickness and crystal structure of the synthesized graphene films.
Conclusions:
- The reported method offers a promising route for scalable, low-temperature synthesis of high-quality graphene.
- This technique allows for precise control over graphene film characteristics, facilitating the realization of its unique properties.
- The findings represent a significant advancement towards the industrial production of graphene for diverse applications.

