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Unconventional magnetization processes and thermal runaway in spin-ice Dy2Ti2O7
D Slobinsky1, C Castelnovo, R A Borzi
1SUPA, School of Physics and Astronomy, University of St Andrews, St Andrews, United Kingdom.
Investigating spin ice Dy2Ti2O7 revealed that below its freezing temperature, magnetization curves deviate from equilibrium. Field-driven monopole excitations cause energy barriers, leading to magnetization steps and sample heating.
Area of Science:
- Condensed Matter Physics
- Magnetism
- Thermodynamics
Background:
- Spin ice materials like Dy2Ti2O7 exhibit complex magnetic behaviors.
- Understanding nonequilibrium dynamics is crucial for characterizing exotic magnetic states.
Purpose of the Study:
- To investigate the nonequilibrium magnetization dynamics of Dy2Ti2O7.
- To correlate magnetization behavior with temperature changes under varying field sweep rates.
Main Methods:
- Magnetization measurements as a function of magnetic field sweep rate.
- Temperature measurements of the sample during magnetization.
Main Results:
- Below the freezing temperature (T(equil)≈600 mK), equilibrium magnetization is not achieved even at slow sweep rates.
- Magnetization curves show flatter initial behavior and sharp steps at higher sweep rates.
- Sharp temperature peaks accompany magnetization steps, indicating inefficient heat dissipation.
Conclusions:
- Nonequilibrium magnetization is governed by energy barriers related to spin flips on filaments.
- Field-driven magnetic monopole excitations dictate the magnetization process.
- Sample heating due to released Zeeman energy can trigger chain reactions.
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