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Updated: Jun 1, 2026
Scale-up Chemical Synthesis of Thermally-activated Delayed Fluorescence Emitters Based on the Dibenzothiophene-S,S-Dioxide Core
Published on: October 24, 2017
Novel Spectrally Stable Saturated Blue-Light-Emitting Poly[(fluorene)-co-(dioctyldibenzothiophene-S,S-dioxide)]s
1Institute of Polymer Optoelectronic Materials and Devices, Key Laboratory of Specially Functional Materials, Ministry of Education, South China University of Technology, Guangzhou 510640, China.
Abstract:
Novel poly[(fluorene)-co-(2,8-dioctyldibenzothiophene-S,S-dioxide-3,7-diyl)]s were synthesized. The octyl group on the 2,8-dioctyldibenzothiophene-S,S-dioxide (DOSO) unit improved the solubility of the polymers and broadened the optical band gap from 2.95 to 3.20 eV as the content of DOSO unit increases. The electroluminescence (EL) spectra of polymers show CIE coordinates around (0.16, 0.07) independent of the ratio of DOSO units in the polymers, owing to the ICT and steric hindrance dual-function. A high efficiency of 3.1 cd · A(-1) (EQE = 3.9%) was obtained with the configuration of ITO/PEDOT:PSS/polymer/Ba/Al. The results indicate that PF-3,7DOSOs could be a promising candidate for saturated blue-emitting polymers with spectral stability and high efficiency.
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