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Flexoelectricity and pattern formation in nematic liquid crystals.

Alexei Krekhov1, Werner Pesch, Agnes Buka

  • 1Physikalisches Institut, Universität Bayreuth, Bayreuth, Germany. alexei.krekhov@uni-bayreuth.de

Physical Review. E, Statistical, Nonlinear, and Soft Matter Physics
|July 7, 2011
PubMed
Summary

We analyzed flexoelectric instability in nematic liquid crystals under alternating electric fields. Unlike static fields, dynamic fields create periodic, bursting stripe patterns (flexodomains).

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Area of Science:

  • Soft Matter Physics
  • Materials Science
  • Liquid Crystal Physics

Background:

  • Flexoelectricity describes the coupling between molecular order and electric fields in liquid crystals.
  • Nematic liquid crystals exhibit unique optical and electrical properties due to their anisotropic molecular alignment.
  • Instabilities in liquid crystals can lead to pattern formation with potential applications in displays and sensors.

Purpose of the Study:

  • To analyze the flexoelectric instability in a planar nematic layer subjected to an alternating electric field.
  • To investigate the dynamic behavior of flexodomains and their transition characteristics.
  • To compare flexoelectric instability with electrohydrodynamic instability in nematics.

Main Methods:

  • Theoretical analysis of the free energy of the nematic layer, including elastic and electric contributions.
  • Investigation of the system's behavior in the limit of low alternating electric field frequencies (ω→0).
  • Comparison of pattern formation under alternating fields versus direct current (dc) fields.

Main Results:

  • Alternating electric fields induce stripe patterns (flexodomains) in the nematic layer.
  • The low-frequency limit (ω→0) of the alternating field case is highly singular.
  • Unlike stationary patterns in the dc case, flexodomains appear as periodic bursts in time at small, finite frequencies.
  • The frequency (ω) acts as a control parameter to tune between flexodomains and convection patterns.

Conclusions:

  • Flexoelectric instability in nematics under alternating fields exhibits unique dynamic behavior, forming time-dependent patterns.
  • The frequency of the alternating electric field is crucial in determining the nature of the observed patterns.
  • Flexodomains represent an equilibrium transition distinct from the nonequilibrium electrohydrodynamic instability.