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Magnetic short-range order in β-Mn(1-x)Co(x).
1ISIS, Rutherford Appleton Laboratory, Harwell Science and Innovation Campus, Didcot OX11 0QX, UK.
Cobalt addition to beta-manganese metal creates a disordered magnetic structure. Both 8c and 12d lattice sites contribute to the magnetic ground state, challenging previous assumptions.
Area of Science:
- Condensed matter physics
- Materials science
- Magnetism
Background:
- Beta-manganese (β-Mn) is an elemental metal with a complex crystal structure.
- Understanding the magnetic properties of β-Mn and its alloys is crucial for materials science applications.
- Previous studies suggested that specific lattice sites in β-Mn were non-magnetic.
Purpose of the Study:
- To investigate the magnetic ground state properties of β-Mn metal alloyed with Cobalt (Co).
- To analyze the magnetic structure and Mn-Mn spin correlations in Co-doped β-Mn.
- To determine the contribution of different lattice sites to the magnetic ground state.
Main Methods:
- Neutron polarization analysis of the diffuse neutron scattering cross-section.
- Reverse Monte Carlo (RMC) procedure for magnetic structure analysis.
- Extraction and analysis of Mn-Mn spin correlations.
Main Results:
- The addition of Co to β-Mn results in a static disordered magnetic structure.
- Medium-range magnetic correlations are observed in the alloy.
- Analysis revealed that both 8c and 12d lattice sites contribute to the magnetic ground state.
- Contrary to prior beliefs, the 8c site is found to be magnetic.
Conclusions:
- Cobalt alloying induces a complex, disordered magnetic state in β-Mn.
- The magnetic ground state arises from contributions from both 8c and 12d lattice sites.
- This finding revises the understanding of magnetism in the β-Mn structure.
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