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Published on: September 23, 2018
Single-layer graphene oxide sheet: a novel substrate for dip-pen nanolithography
1School of Materials Science and Engineering, Nanyang Technological University, 50 Nanyang Avenue, Singapore 639798, Singapore.
Summary
Graphene oxide sheets serve as a novel substrate for dip-pen nanolithography. This technique enables simultaneous patterning of cobalt chloride on graphene oxide and silicon dioxide for carbon nanotube growth.
Area of Science:
- Materials Science
- Nanotechnology
- Surface Chemistry
Background:
- Graphene oxide (GO) is a promising material for nanoscale applications.
- Dip-pen nanolithography (DPN) is a versatile technique for patterning surfaces.
- Controlled growth of carbon nanotubes (CNTs) requires precise surface patterning.
Purpose of the Study:
- To investigate the use of graphene oxide (GO) as a substrate for dip-pen nanolithography (DPN).
- To demonstrate the simultaneous patterning of CoCl(2) on GO and SiO(2) substrates.
- To explore the application of DPN-patterned substrates for the growth of various carbon nanotube structures.
Main Methods:
- Transferring graphene oxide (GO) sheets onto SiO(2) substrates using the Langmuir-Blodgett technique.
- Utilizing dip-pen nanolithography (DPN) to pattern cobalt chloride (CoCl(2)) onto the GO/SiO(2) surface.
- Growing different structured carbon nanotubes (CNTs) on the patterned substrates.
Main Results:
- Graphene oxide (GO) proved to be a suitable and novel substrate for DPN.
- CoCl(2) was successfully patterned simultaneously on both GO and exposed SiO(2) areas.
- The patterned substrates facilitated the growth of diverse carbon nanotube structures.
Conclusions:
- Graphene oxide (GO) is an effective substrate for dip-pen nanolithography (DPN).
- DPN on GO/SiO(2) enables precise, simultaneous patterning for controlled nanomaterial synthesis.
- This approach offers a new pathway for fabricating structured carbon nanotubes.

