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Updated: May 29, 2026

Unraveling Entropic Rate Acceleration Induced by Solvent Dynamics in Membrane Enzymes
Published on: January 16, 2016
Nicholas Boekelheide1, Romelia Salomón-Ferrer, Thomas F Miller
1Division of Chemistry and Chemical Engineering, California Institute of Technology, 1200 East California Boulevard, Mail Code 127-72, Pasadena, CA 91125, USA.
Enzyme vibrations play a minimal role in hydride transfer. Protein fluctuations statistically gate the reaction barrier, rather than directly influencing it through nonlocal dynamics.
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