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Updated: May 26, 2026

Direct Imaging of Laser-driven Ultrafast Molecular Rotation
Published on: February 4, 2017
Generation of soft x-ray and water window harmonics using a few-cycle, phase-locked, optical parametric chirped-pulse
Nobuhisa Ishii1, Shunsuke Adachi, Yutaka Nomura
1Institute for Solid State Physics, University of Tokyo, Kashiwanoha 5-1-5, Kashiwa, Chiba 277-8581, Japan. ishii@issp.u‐tokyo.ac.jp
Abstract:
Multimillijoule, few-cycle, carrier-envelope-phase (CEP)-locked, near-IR pulses at 750 nm from an optical parametric chirped-pulse amplifier are applied to the generation of CEP-dependent, soft x-ray high harmonics around the boron K-edge at 188 eV. The dependence on the CEP manifests the phase coherence of high harmonics preserved in the highest-photon energy ever reported. Multimillijoule optical pulses also allow the extension of the cutoff energy up to 325 eV, exceeding the carbon K-edge of the water window. However, in this spectral range, the CEP dependence of harmonic spectra is not observed, suggesting the degradation of temporal coherence due to the heavy ionization of helium atoms.
