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Self-assembled bilayers on indium-tin oxide (SAB-ITO) electrodes: a design for chromophore-catalyst photoanodes
Christopher R K Glasson1, Wenjing Song, Dennis L Ashford
1Department of Chemistry, University of North Carolina, Chapel Hill, North Carolina 27599-3290, USA.
Inorganic Chemistry
|August 4, 2012
Abstract:
A novel approach for creating assemblies on metal oxide surfaces via the addition of a catalyst overlayer on a chomophore monolayer derivatized surface is described. It is based on the sequential self-assembly of a chromophore, [Ru(bpy)(4,4'-(PO(3)H(2)bpy)(2))](2+), and oxidation catalyst, [Ru(bpy)(P(2)Mebim(2)py)OH(2)](2+), pair, resulting in a spatially separated chromophore-catalyst assembly.
