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Asymmetric thermal line shape broadening in a gapped 3D antiferromagnet: evidence for strong correlations at finite
D L Quintero-Castro1, B Lake, A T M N Islam
1Helmholtz-Zentrum Berlin für Materialien und Energie, Berlin, Germany. diana.quintero_castro@helmholtz-berlin.de
Abstract:
It is widely believed that magnetic excitations become increasingly incoherent as the temperature is raised due to random collisions which limit their lifetime. This picture is based on spin-wave calculations for gapless magnets in 2 and 3 dimensions and is observed experimentally as a symmetric Lorentzian broadening in energy. Here, we investigate a three-dimensional dimer antiferromagnet and find unexpectedly that the broadening is asymmetric-indicating that far from thermal decoherence, the excitations behave collectively like a strongly correlated gas. This result suggests that a temperature activated coherent state of quasiparticles is not confined to special cases like the highly dimerized spin-1/2 chain but is found generally in dimerized antiferromagnets of all dimensionalities and perhaps gapped magnets in general.
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