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Updated: May 16, 2026

Experimental Methods for Spin- and Angle-Resolved Photoemission Spectroscopy Combined with Polarization-Variable Laser
Published on: June 28, 2018
Resonant photoemission and spin polarization of Co(1-x)Fe(x)S(2)
Xin Zhang1, Ning Wu, Michael Manno
1Nebraska Center for Materials and Nanoscience, Department of Physics and Astronomy, University of Nebraska-Lincoln, 68588-0299, USA.
Abstract:
The valence band occupied state electronic structure of Co(1-x)Fe(x)S(2) in the region of the Fe/Co 3d bands has been investigated using photoemission and spin-polarized photoemission. As measured by using spin-polarized ultraviolet photoemission, the surface Fermi level spin polarization of Co(1-x)Fe(x)S(2) thin films at 50 K, specifically at x = 0, 0.05, 0.10 and 0.15, was found to be much reduced compared to that of the bulk. The spin polarization nonetheless increases with Fe concentration. The resonant photoemission spectroscopy provides evidence that S bands have a strong resonance at the photon energy corresponding to the Co 2p core level, indicating strong hybridization between Co and S bands in Co(1-x)Fe(x)S(2) (at small x). Similar evidence exists for Fe hybridization with the S bands.
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