Related Experiment Video
Updated: May 15, 2026

Generation and Coherent Control of Pulsed Quantum Frequency Combs
Published on: June 8, 2018
Generation of single-cycle mid-infrared pulses via coherent synthesis
Fen Ma1, Hongjun Liu, Nan Huang
1State Key Laboratory of Transient Optics and Photonics, Xi’an Institute of Optics and Precision Mechanics, Chinese Academy of Science (CAS), Xi'an, 710119, China.
Abstract:
A new approach for the generation of single-cycle mid-infrared pulses without complicated control systems is proposed, which is based on direct coherent synthesis of two idlers generated by difference frequency generation (DFG) processes. It is found that the waveform of synthesized pulses is mainly determined by the spectra superposition, the carrier-envelope phase (CEP) difference, the relative timing and the chirp ratio between the idlers. The influences of these parameters on the synthesized waveform are also numerically calculated and analyzed via second-order autocorrelation, which offers general guidelines for the waveform optimization. The single-cycle synthesized mid-infrared pulses, which are centered at 4233 nm with the spectrum spanning from 3000 nm to 7000 nm, are achieved by carefully optimizing these parameters. The single-cycle mid-infrared laser source presents the possibility of investigating and controlling the strong field light-matter interaction.
Related Concept Videos
Infrared (IR) Spectroscopy: Overview
Different compounds display unique properties due to their...
IR Spectroscopy: Molecular Vibration Overview
Stretching vibrations are vibrational motions that occur along the bond line, changing the bond length or distance between two bonded atoms. They are further distinguished as symmetric or asymmetric. In symmetric stretching, the...
NMR Spectrometers: Radiofrequency Pulses and Pulse Sequences
IR Spectrometers
IR Absorption Frequency: Hybridization
Among the sp, sp2, and sp3 hybridized orbitals, sp orbitals have the maximum s character (50%). Consequently, the electrons are held more closely to the nucleus, resulting in stronger and shorter C–H bonds that stretch at a...
Applications of IR Spectroscopy: Overview
