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Related Experiment Video

Updated: May 15, 2026

Focused Ion Beam Fabrication of LiPON-based Solid-state Lithium-ion Nanobatteries for In Situ Testing
10:58

Focused Ion Beam Fabrication of LiPON-based Solid-state Lithium-ion Nanobatteries for In Situ Testing

Published on: March 7, 2018

Self-limiting lithiation in silicon nanowires.

Xiao Hua Liu1, Feifei Fan, Hui Yang

  • 1Center for Integrated Nanotechnologies-CINT, Sandia National Laboratories, Albuquerque, New Mexico 87185, USA. lxhua99@gmail.com

ACS Nano
|January 1, 2013
PubMed
Summary

Lithiation kinetics in silicon nanowires for lithium-ion batteries are self-limiting due to stress. This study measures nanoscale growth rates, impacting high-performance battery design.

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Area of Science:

  • Materials Science
  • Electrochemistry
  • Nanotechnology

Background:

  • Lithium-ion battery (LIB) performance relies on electrode kinetics.
  • Silicon anodes offer high capacity but have unclear lithiation mechanisms.

Purpose of the Study:

  • Investigate the lithiation kinetics in individual silicon nanowires.
  • Clarify the reaction and diffusion processes of lithium in silicon.

Main Methods:

  • Combined experimental and theoretical approach.
  • In situ transmission electron microscopy (TEM) to observe lithiation.
  • Measurement of amorphous Li(x)Si layer growth rate.

Main Results:

  • Quantified the nanoscale growth kinetics of lithiated silicon.

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Last Updated: May 15, 2026

Focused Ion Beam Fabrication of LiPON-based Solid-state Lithium-ion Nanobatteries for In Situ Testing
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Published on: March 7, 2018

Monolayer Contact Doping of Silicon Surfaces and Nanowires Using Organophosphorus Compounds
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  • Observed self-limiting lithiation behavior in silicon nanowires.
  • Identified lithiation-induced stress as a retardation factor.

    • Conclusions:

    • Stress significantly impacts lithiation kinetics in silicon anodes.
    • Understanding these kinetics is crucial for designing high-capacity, high-rate LIBs.
    • Findings guide nanostructure development for advanced LIBs.