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Soft X-ray spectromicroscopy using ptychography with randomly phased illumination.

A M Maiden1, G R Morrison, B Kaulich

  • 1Department of Electronic and Electrical Engineering, University of Sheffield, Sheffield S1 3JD, UK.

Nature Communications
|April 12, 2013
PubMed
Summary
This summary is machine-generated.

This study introduces a new ptychography method using a randomly phased X-ray probe to reduce diffraction data dynamic range. This technique enables robust imaging and chemical sensitivity in soft X-ray spectromicroscopy.

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Area of Science:

  • Diffractive imaging
  • X-ray microscopy
  • Spectromicroscopy

Background:

  • Ptychography retrieves sample transmission function and probe.
  • Large dynamic range of diffraction data is an experimental challenge.
  • Soft X-ray spectromicroscopy requires chemical sensitivity.

Purpose of the Study:

  • To develop a novel ptychographic experiment to reduce diffraction data dynamic range.
  • To demonstrate robust image reconstruction with weak scatter.
  • To showcase chemical sensitivity in soft X-ray spectromicroscopy.

Main Methods:

  • Utilized a randomly phased X-ray probe in a ptychographic setup.
  • Performed ptychographic reconstructions at X-ray energies around the iron L absorption edge.
  • Acquired and analyzed diffraction patterns with reduced dynamic range.

Main Results:

  • Successfully reduced the dynamic range of recorded diffraction patterns.
  • Achieved reliable and robust image reconstruction, even with weak specimen scatter.
  • Demonstrated chemical sensitivity without optical refocusing.
  • Phase and modulus signals were in perfect registration, providing complementary information.

Conclusions:

  • The novel ptychographic method effectively reduces diffraction data dynamic range.
  • This approach enhances robustness and enables chemical sensitivity in soft X-ray spectromicroscopy.
  • The phase signal offers complementary, sensitive information for analyzing local chemical environments.