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Updated: May 11, 2026

10:52
Direct Imaging of Laser-driven Ultrafast Molecular Rotation
Published on: February 4, 2017
Bounce-by-bounce cavity ring-down spectroscopy: femtosecond temporal imaging
A M Shaw1, R N Zare, C V Bennett
1Department of Chemistry, Stanford University, Stanford, CA 94305-5080, USA.
Abstract:
A time microscope (100× magnification) allows light pulses exiting an optical cavity to be viewed one at a time. A linearly chirped Gaussian pulse is mixed in a nonlinear crystal with the dispersed input waveform; the up-converted light is sent onto an output dispersive network. The resulting temporal image is recorded both with a streak camera and with a spectrometer.

