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Updated: May 9, 2026

10:52
Direct Imaging of Laser-driven Ultrafast Molecular Rotation
Published on: February 4, 2017
Ultrahigh contrast from a frequency-doubled chirped-pulse-amplification beamline
David Hillier1, Colin Danson, Stuart Duffield
1Atomic Weapons Establishment plc, Reading, Berkshire, UK. david.hillier@awe.co.uk
Applied Optics
|July 12, 2013
Summary
This study demonstrates high-energy, frequency-doubled laser pulses using a chirped-pulse amplification (CPA) beamline. Efficient second-harmonic generation produced over 100 Joules in a subpicosecond pulse at 527 nm.
Area of Science:
- Laser physics
- Nonlinear optics
- High-energy lasers
Background:
- Chirped-pulse amplification (CPA) is a technique for amplifying ultrashort laser pulses.
- Frequency doubling (second-harmonic generation) converts laser light to half its wavelength, often with nonlinear crystals.
- High-energy, short-pulse lasers are crucial for research in fields like inertial confinement fusion and materials science.
Purpose of the Study:
- To describe the frequency-doubled operation of a high-energy CPA beamline.
- To achieve efficient second-harmonic generation (SHG) at high laser energies.
- To characterize the performance of the 527 nm laser pulse output.
Main Methods:
- Utilized a high-energy chirped-pulse amplification (CPA) beamline.
- Employed type-I second-harmonic generation (SHG) with a potassium dihydrogen phosphate (KDP) crystal.
- Conducted experiments across a range of laser energies.
Main Results:
- Achieved efficient type-I second-harmonic generation (SHG) using a 3 mm thick, 320 mm aperture KDP crystal.
- Generated laser pulses exceeding 100 Joules (J) at 527 nm.
- Produced subpicosecond pulses with a high power contrast ratio of 10^14.
Conclusions:
- Demonstrated successful frequency-doubled operation of a high-energy CPA system.
- Validated the use of KDP crystals for efficient SHG in high-power laser systems.
- The achieved pulse parameters (energy, duration, contrast) are suitable for demanding applications.
