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Wavelength-tunable spasing in the visible.

Xiangeng Meng1, Alexander V Kildishev, Koji Fujita

  • 1Department of Material Chemistry, Graduate School of Engineering, Kyoto University , Katsura, Nishikyo-ku 615-8510, Kyoto, Japan.

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|August 7, 2013
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Summary

Researchers achieved room-temperature surface plasmon amplification by stimulated emission of radiation (SPASER) in the visible range. This breakthrough overcomes dissipative losses using gold nanorods and laser dyes, enabling tunable nanoscale coherent optical fields.

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Area of Science:

  • Plasmonics and Nanophotonics
  • Materials Science
  • Quantum Optics

Background:

  • Surface plasmon amplification by stimulated emission of radiation (SPASER) is crucial for nanoscale coherent optical fields.
  • Realizing visible-range SPASERs is challenging due to significant dissipative losses in plasmonic systems.

Purpose of the Study:

  • To demonstrate room-temperature SPASER emission in the visible range.
  • To overcome dissipative losses in plasmon nanocavities.
  • To achieve tunable SPASER emission wavelengths.

Main Methods:

  • Utilized gold nanorods as plasmon nanocavities to support longitudinal surface plasmon modes.
  • Employed laser dyes to provide optical gain, compensating for plasmon losses.
  • Adjusted dye type and doping concentration to tune emission characteristics.

Main Results:

  • Achieved room-temperature SPASER emission by amplifying surface plasmon modes in gold nanorods.
  • Demonstrated tunable emission from 562 to 627 nm by selecting specific organic dyes and doping levels.
  • Narrowed the spectral line width of the SPASER emission to 5-11 nm.

Conclusions:

  • Successfully demonstrated a room-temperature visible-range SPASER by compensating plasmon losses with optical gain.
  • The developed method offers a versatile approach for achieving SPASERs across extended wavelength regimes.
  • This work paves the way for advanced nanoscale optical applications requiring coherent light sources.