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Ultrasmooth metallic films with buried nanostructures for backside reflection-mode plasmonic biosensing.

Nathan C Lindquist1, Timothy W Johnson, Jincy Jose

  • 1Laboratory of Nanostructures and Biosensing, Department of Electrical and Computer Engineering, University of Minnesota, Minneapolis, MN 55455 USA.

Annalen Der Physik
|October 26, 2013
PubMed
Summary

We developed a novel plasmonic device with buried nanostructures on ultrasmooth surfaces for advanced biosensing. This architecture enables sensitive detection of opaque liquids using backside reflection-mode imaging.

Keywords:
Atomically Flat Gold FilmBiosensingGrating CouplersNanolithographyNanostructuresPlasmonicsSurface Plasmon Resonance (SPR)Template Stripping

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Area of Science:

  • Nanophotonics
  • Plasmonics
  • Biosensing

Background:

  • Traditional surface plasmon resonance (SPR) sensors face limitations with opaque or scattering samples.
  • Achieving ultrasmooth surfaces is crucial for high-performance plasmonic devices.

Purpose of the Study:

  • To introduce a new plasmonic device architecture featuring buried nanostructures.
  • To demonstrate its utility for biosensing applications, particularly with challenging liquid samples.

Main Methods:

  • Utilizing template-stripping techniques to create ultrathin gold films (<5 Å roughness).
  • Optically coupling these films to buried metallic gratings, rings, or nanodots.
  • Implementing a backside, reflection-mode geometry for decoupled optical and fluidic access.

Main Results:

  • Demonstrated a prototypical device with buried linear plasmonic gratings for biosensing.
  • Achieved high sensitivity and decoupled optical access, similar to prism-based SPR.
  • Enabled sensing with opaque and highly scattering liquids.
  • Showcased benefits of nanoplasmonics like spectral tunability and wide-field imaging.

Conclusions:

  • The new architecture offers a versatile platform for biosensing with enhanced capabilities.
  • The design is suitable for various applications including nanophotonic waveguides and spectroscopy.
  • Ultrasmooth surfaces with buried nanostructures represent a significant advancement in plasmonic device design.